Batteries, Vol. 12, Pages 45: Coupling Model and Early-Stage Internal Short Circuits Fault Diagnosis for Gel Electrolyte Lithium-Ion Batteries

Batteries doi: 10.3390/batteries12020045

Authors:
Liye Wang
Jinlong Wu
Chunxiao Ma
Xianzhong Sun
Lifang Wang
Chenglin Liao

This paper presents a method for modeling and predicting ISC in gel-electrolyte lithium-ion batteries, addressing critical safety concerns in electric vehicles. While gel-electrolytes are highlighted for their superior stability and performance advantages over liquid-electrolytes, they remain susceptible to IISC due to factors such as dendrite formation or mechanical stress. This study provides a detailed analysis of the unique ISCs mechanism in gel-electrolytes, emphasizing the differences between gel-electrolyte and liquid-electrolyte batteries in terms of ion transport dynamics and thermal performance. Based on these characteristics, an electrochemical–thermal–ISC coupling model was developed, and an external short-circuit resistance test was conducted to validate the model’s accuracy. By simulating various ISC states using the coupling model, a comprehensive dataset of battery ISC parameters was obtained, encompassing voltage, current, temperature, SOC, capacity loss, and internal resistance. ISC prediction models were subsequently developed using BP, CNN, and LSTM networks, with a comparative analysis of their prediction accuracy. This research advances the ISC prediction framework for gel-electrolyte batteries and demonstrates the potential of CNN-based models to achieve higher accuracy in fault prediction. Accurate ISC prediction is crucial for ensuring safe battery operation in electric vehicles.

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